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    Energy Transfer from Colloidal Nanocrystals into Si Substrates Studied via Photoluminescence Photon Counts and Decay Kinetics

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    Date
    2013-08-16
    Author
    Nguyen, H. M.
    Seitz, Oliver
    Gartstein, Yuri N.
    Chabal, Yves J.
    Malko, Anton V.
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    Abstract
    Abstract
    We use time-resolved photoluminescence (PL) kinetics and PL intensity measurements to study the decay of photoexcitations in colloidal CdSe/ZnS nanocrystals grafted on SiO₂ - Si substrates with a wide range of the SiO₂ spacer layer thicknesses. The salient features of experimental observations are found to be in good agreement with theoretical expectations within the framework of modification of spontaneous decay of electric-dipole excitons by their environment. Analysis of the experimental data reveals that energy transfer (ET) from nanocrystals into Si is a major enabler of substantial variations in decay rates, where we quantitatively distinguish contributions from nonradiative and radiative ET channels. We demonstrate that time-resolved PL kinetics provides a more direct assessment of ET, while PL intensity measurements are also affected by the specifics of the generation and emission processes.
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    http://hdl.handle.net/10735.1/3900
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    • Chabal, Yves J.
    • Gartstein, Yuri N.
    • Malko, Anton V.
    • NSM Staff-Student Research

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