Enhanced Shape Stability of Pd-Rh Core-Frame Nanocubes at Elevated Temperature: In Situ Heating Transmission Electron Microscopy

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Abstract

Shape stability of Pd-Rh core-frame nanocubes was studied by in situ heating transmission electron microscopy. Pd-Rh nanocubes could maintain cubic shape at elevated temperature compared with pure Pd. The surface diffusion process of Rh onto {100} side surfaces is believed to postpone the degradation to higher temperature.

Description

Includes supplementary material.

Keywords

Nanocubes, Rhodium alloys, Palladium alloys, Electron microscopy

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"This work was supported by AOARD-AFOSR (FA2385-10-1-4066) and the World Class University Program (by MEST through NRF (R31-10026)). The synthesis work was supported in part by a grant from the NSF (DMR-1215034) and start-up funds from Georgia Institute of Technology."

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©2013 The Royal Society of Chemistry. This article may not be further made available or distributed.

Citation

Lu, N., J. Wang, S. Xie, Y. Xia, et al. 2013. "Enhanced shape stability of Pd-Rh core-frame nanocubes at elevated temperature: In situ heating transmission electron microscopy." Chemical Communications 49: 1806-11808.

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